Ionic motion and Disordered Structure in the Rotator Phase of Butylammonium Chloride Studied by Temperature Dependences

نویسندگان

  • Mineyuki Hattori
  • Yoshito Onoda
  • Tomoki Erata
  • Masakazu Hattori
  • Hiroshi Ohki
  • Ryuichi Ikeda
چکیده

Temperature dependences of 35C1 and 2H quadrupole coupling constants and 35C1 NM R spin-lat­ tice relaxation times in polycrystalline samples were measured in the rotator phase of the butylam­ monium chlorides C4H 9N H 3C1 and C4H 9N D 3C1, obtainable above the phase transition tempera­ ture of 241 K. A rapid decrease of the quadrupole coupling constants of both nuclei upon heating is attributed to increasing dynamic disorder formed around the polar head. The presence of self-diffussion of C P ions was revealed from the spin-spin relaxation time and resonance line-width in single crystals, and confirmed by measuring the dc electrical conductivity.

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تاریخ انتشار 2013